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金属有机活性中间体导向的催化反应及机理研究
2015-09-30 09:43   (浏览次数: ) [文字大小: ]
活动地点: 闵行校区化学A楼526演讲厅
活动时间: 2015-10-09 16:00:00

[责任编辑]刘怡婷 [信息提供]化学化工学院

报告主题:金属有机活性中间体导向的催化反应及机理研究

报告人:黄汉民 研究员,兰州化学物理研究所

报告时间:2015年10月9日(周五)16:00

报告地点:闵行校区化学A楼526演讲厅

邀请人:张万斌教授
    Prof. Wanbin Zhang

报告人简介:

  黄汉民,男,1974年出生,研究员,博士生导师,羰基合成与选择氧化国家重点实验室常务副主任,所学术委员会委员。2003年于中科院大连化学物理研究所获得有机化学博士学位,2004年至2008年在日本名古屋大学物质科学国际研究中心从事博士后研究,期间获得JSPS-Fellow基金支持。2008年4月起在兰州化学物理研究所开始从事独立研究工作,建立了有机合成研究小组,并入选中科院“百人计划”。主要研究领域为导向有机合成的金属有机化学研究,在不对称催化和惰性键的选择性活化方面开展研究工作。近年来,作为第一作者或通讯作者已在Chem. Rev; J. Am. Chem. Soc.; Angew. Chem. Int. Ed.; Chem. Eur. J.;Org. Lett.;Chem.Comm.; J. Org. Chem.等刊物上发表研究论文70多篇,其中SCI-I区(IF>10)共15篇,被引用1500多次。授权中国专利2项,美国专利1项,日本专利1项;申请中国专利10多项。相关研究工作分别被美国化学会的《化学与工程新闻》(Chemical & Engineering News)、《自然》(Nature)期刊的子刊(Nature Chemical Biology)、专业评论期刊Synform和Synfacts作为亮点进行评论和转载。2012年获得国家自然科学基金“优秀青年基金”的资助,2013年中科院“百人计划”结题为优秀,并获得第二届中国均相催化青年奖,2015年度中国科学院优秀研究生指导教师奖。

代表论文:

Guiping Qin, Lixin Li, Jiawen Li, and Hanmin Huang*, Palladium-Catalyzed Formal Insertion of Carbenoids into Aminals via C-N Bond Activation, J. Am. Chem. Soc. 2015, 137, DOI: 10.1021/jacs.5b08476, ASAP.
Hui Yu, Guoying Zhang, and Hanmin Huang*, Palladium-Catalyzed Dearomative Cyclocarbonylation via C-N Bond Activation, Angew. Chem. Int. Ed. 2015, 54, 10912-10916.
Guoying Zhang, Bao Gao, and Hanmin Huang*, Palladium-Catalyzed Hydroaminocarbonylation of Alkenes with Amines: A Strategy to Overcome Basicity-Barrier Imparted by Aliphatic Amines, Angew. Chem. Int. Ed. 2015, 54, 7657-7661.
Yinjun Xie, Shengmei Guo, Longmin Wu, Chungu Xia, and Hanmin Huang*, Metal Bridging for Directing and Accelerating Electron Transfer as Exemplified by Harnessing the Reactivity of AIBN, Angew. Chem. Int. Ed. 2015, 54, 5900-5904.
Lei Yang, and Hanmin Huang*, Transition-Metal-Catalyzed Direct Addition of Unactivated C−H Bonds to Polar Unsaturated Bonds, Chem. Rev. 2015, 115, 3468-3517.
Jianhua Hu, Yinjun Xie, and Hanmin Huang*, Palladium-Catalyzed Insertion of an Allene into an Aminal: Aminomethylamination of Allenes via C-N Bond Activation, Angew. Chem. Int. Ed. 2014. 53, 7272-7276.
Yinjun Xie, Jianhua Hu, Pan Xie, Bo Qian, and Hanmin Huang*, Palladium-Catalyzed Difunctionalization of Enol Ethers to Amino Acetals with Aminals and Alcohols, J. Am. Chem. Soc. 2013, 135, 18327-18330.
Guoying Zhang, Lei Yang, Yanyu Wang, Yinjun Xie, and Hanmin Huang*, An Efficient Rh/O2 Catalytic System for Oxidative C-H Activation/Annulation: Evidence for Rh(I) to Rh(III) Oxidation by Molecular Oxygen, J. Am. Chem. Soc. 2013, 135, 8850-8853.
Yinjun Xie, Jianhua Hu, Yanyu Wang, Chungu Xia, and Hanmin Huang*, Palladium-Catalyzed Vinylation of Aminals with Simple Alkenes: A New Strategy to Construct Allylamines. J. Am. Chem. Soc. 2012, 134, 20613-20616.
Pan Xie, Yinjun Xie, Bo Qian, Han Zhou, Chungu Xia, and Hanmin Huang*, Palladium-Catalyzed Oxidative Carbonylation of Benzylic C-H Bonds via Nondirected C(sp3)-H Activation. J. Am. Chem. Soc. 2012, 134, 9902-9905.
Dengjian Shi, Yinjun Xie, Han Zhou, Chungu Xia, and Hanmin Huang*, A Highly Diastereo- and Enantioselective Reaction for Constructing Functionalized Cyclohexanes: Six Contiguous Stereocenters in one Step. Angew. Chem. Int. Ed. 2012, 51, 1248-1251. (Highlight by Chemical & Engineering News、Nature Chemical Biology和Synform).
Yinjun Xie, Yingwei Zhao, Bo Qian, Lei Yang, Chungu Xia, and Hanmin Huang*, Enantioselective N-H Functionalization of Indole with α,β-Unsaturated γ-Lactams Catalyzed by Brønsted Acids. Angew. Chem. Int. Ed. 2011, 50, 5682-5686. (Highlight by Synfacts, 同时被评为2011年Angew. Chem. Int. Ed.下载量最多的25篇之一,排在第9位)。
Shengmei Guo, Yinjun Xie, Xinquan Hu, Chungu Xia, and Hanmin Huang*, Diastereo- and Enantioselective Catalytic Tandem Michael Addition/Mannich Reaction: Access to Chiral Isoindolinones and Azetidines with Multiple Stereocenters. Angew. Chem. Int. Ed. 2010, 49, 2728-2731.( Highlight by Synfacts).
Bo Qian, Shengmei Guo, Jianping Shao, Qiming Zhu, Lei Yang, Chungu Xia*, and Hanmin Huang*, Palladium-Catalyzed Benzylic Addition of 2-Methyl Azaarenes to N-Sulfonyl Aldimines via C-H Bond Activation. J. Am. Chem. Soc. 2010, 132, 3650-3651.
Hanmin Huang, Tomoko Okuno, Kazuomi Tsuda, Masahiro Yoshimura, Masato Kitamura* “Enantioselective Hydrogenation of Aromatic Ketones Catalyzed by Ru Complexes of Goodwin-Lions-type sp2N/sp3N hybrid Ligands R-BINAN-R΄-Py” J. Am. Chem. Soc. 2006, 128, 8716-8717.


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